Coherent peaks and minimal probing depth in photoemission spectroscopy of Mott-Hubbard systems.

نویسندگان

  • G Panaccione
  • M Altarelli
  • A Fondacaro
  • A Georges
  • S Huotari
  • P Lacovig
  • A Lichtenstein
  • P Metcalf
  • G Monaco
  • F Offi
  • L Paolasini
  • A Poteryaev
  • O Tjernberg
  • M Sacchi
چکیده

We have measured hard x-ray photoemission spectra of pure vanadium sesquioxide (V(2)O(3)) across its metal-insulator transition. We show that, in the metallic phase, a clear correlation exists between the shakedown satellites observed in the vanadium 2p and 3p core-level spectra and the coherent peak measured at the Fermi level. Comparing experimental results and dynamical mean-field theory calculations, we estimate the Hubbard energy U in V(2)O(3) (4.20+/-0.05 eV). From our bulk-sensitive photoemission spectra we infer the existence of a critical probing depth for investigating electronic properties in strongly correlated solids.

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Bulk- and surface-sensitive high-resolution photoemission study of two mott-hubbard systems: SrVO3 and CaVO3.

We study the electronic structure of Mott-Hubbard systems SrVO3 and CaVO3 with bulk and surface-sensitive high-resolution photoemission spectroscopy, using a vacuum ultraviolet laser, synchrotron radiation, and a discharge lamp (hv = 7-21 eV). A systematic suppression of the density of states (DOS) within approximately 0.2 eV of the Fermi level (EF) is found on decreasing photon energy, i.e., o...

متن کامل

Phenomenological Modeling of Photoemission Spectra in Strongly Correlated Electron Systems

A phenomenological approach is presented that allows one to model, and thereby interpret, photoemission spectra of strongly correlated electron systems. A simple analytical formula for the self-energy is proposed. This self-energy describes both coherent and incoherent parts of the spectrum (quasiparticle and Hubbard peaks, respectively). Free parameters in the expression are determined by fitt...

متن کامل

Tuning the Mott transition in a Bose-Einstein condensate by multiple photon absorption.

We study the time-dependent dynamics of a Bose-Einstein condensate trapped in an optical lattice. Modeling the system as a Bose-Hubbard model, we show how applying a periodic driving field can induce coherent destruction of tunneling. In the low-frequency regime, we obtain the novel result that the destruction of tunneling displays extremely sharp peaks when the driving frequency is resonant wi...

متن کامل

Direct observation of the mass renormalization in SrVO3 by angle resolved photoemission spectroscopy.

Band dispersions and Fermi surfaces of the three-dimensional Mott-Hubbard system SrVO3 are directly observed by angle-resolved photoemission spectroscopy. An observed spectral weight distribution near the Fermi level (E(F)) shows cylindrical Fermi surfaces as predicted by band-structure calculations. By comparing the experimental results with calculated surface electronic structures, we conclud...

متن کامل

Strong- and weak-coupling mechanisms for pseudogap in electron-doped cuprates

Using the two-particle self-consistent approach and cluster perturbation theory for the two-dimensional t-t′-t′′-U Hubbard model, we discuss weakand strong-coupling mechanisms for the pseudogap observed in recent angle resolved photoemission spectroscopy on electron-doped cuprates. In the case of the strong-coupling mechanism, which is more relevant near half-filling, the pseudogap can be mainl...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

عنوان ژورنال:
  • Physical review letters

دوره 97 11  شماره 

صفحات  -

تاریخ انتشار 2006